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J. Soc. Cosmet. Chem., 29, 307-322 (May 1978) SYNTHESEN IN DER ISOCAMPHANREIHE, Clber den Geruchseindruck von Isocamphanderivaten IX. * G. BUCHBAUER* * und M. WILTSCHKO* * * Synopsis -- A total of 55 isocamphane derivatives was studied in order to establish a correlation between the shape of the molecule and xts odor as postulated by the theory of Arnoore. The molecules were measured by use of the shadow matching method and compared with cxneole, the camphoraceous odor standard. The agreement of the results of these measurements with other molecular parameters, e.g. boxhng point, was also examined. Isocamphane derivatives with spherical shape exhibit a distinct camphoraceous odor, and this charcteristic is reduced as the asymmetry of the isocamphane molecule increases. Nach J. E. Amoore [1} ist die Gestalt bzw. die Raumerfillung eines Molekills der wesentliche Faktor fir die Entstehung der verschiedenen Geruchseindrficke. Wenn nun einige Molekile einen gleichen oder •ihnlichen Geruch hervorrufcn, so missen sic nach dieser Theorie daher auch gleiche oder •ihnliche Gestalt haben und von anderen Molekilen mit anderen Gerichen in der Gestalt mehr oder minder deutlich ver- schieden sein. Es erschien daher interessant, eine gr6gere Anzahl von Isocamphanverbindungen, die entweder als Riechstoffe selbst oder als Zwischenprodukte bei der Synthese von Riechstoffen von potentidler * 8. Mitteiltmg, G. Buchbauer und E. Klissenbauer, Mh. Chem., •m Druck. ** Pharmazeutisch-Chemisches Institut der Universxtat Wien, A 1090 Wien, Wahringer- stral•e 10. * * * Teil der Diplomarbeit yon M. Wiltschko, Universitat Wien, 1977. Der Firma Dragoco, Wien-Liesing, danken wir ftir wohlwollende Unterstfitztmg. 307